| Aaron Himelstein | Specialist Cameron Klein |
| Aaron Taylor-Johnson | Pietro Maximoff / Quicksilver |
| Abigail Marlowe | S.H.I.E.L.D. Tech |
| Adam Caroselli | Reporter |
| Adetokumboh M'Cormack | French Radio Pirate |
| Adrian Denzel | DC Pedestrian |
| Al Sotto | Museum Guest |
| Alan Dale | Councilman Rockwell |
| Alan Christopher Davis | National Mall Jogger |
| Allan Chanes | Launch Tech #2 |
| Alvin J. Frazier II | S.H.I.E.L.D. Tech Agent |
| Amanda Burry | Museum Patron |
| Andrew Constantini | WW2 Russian Soldier |
| Andrew Kiser | Museum Guest |
| Andy Martinez Jr. | Capitol Hill Police |
| Andy Tatarko | DC Pedestrian |
| Angela Russo-Otstot | Garcia |
| Ann Russo | Strike Agent |
| Anne Grimenstein | Committee Member |
| Annette Lawless | S.H.I.E.L.D. Agent |
| Anthony Mackie | Sam Wilson / Falcon |
| Arne Sagnes | Museum Guest |
| Aswan Harris | S.H.I.E.L.D. Security |
| Ben Atkins | Military Veteran |
| Bernard White | Councilman Singh |
| Bernard Zilinskas | Com Tech #2 |
| Beshoy Hanna | Victim |
| Bill Kennedy | DC Cop |
| Brandon Singleton | Museum Tourist |
| Branka Katić | Renata |
| Brenda Sampson | Museum Patron |
| Brent Reichert | S.H.I.E.L.D. Agent |
| Brian Duffy | French Pirate #2 |
| Brian Hartong | S.H.I.E.L.D. Agent |
| Brian R. Moore | DC Cop |
| Britney Meeks | Museum Visitor |
| Brittany Buck | Mall Patron |
| Brittany Tyjeski | Tech Agent |
| Bryan Geary | Museum Guest |
| Bryan Pixler | Museum Security Guard |
| Bryon Tobin | Mall Pedestrian |
| Callan Mulvey | Jack Rollins |
| Carlos Lopez Jr. | SWAT Member |
| Carmen Dee Harris | Mall Patron |
| Carmen Gangale | Mall Patron |
| Chad Daubenmire | S.H.I.E.L.D. Agent |
| Chad Todhunter | Charlie Weapons Tech |
| Charlene May | Hostage |
| Charles Wittman | Capitol Hill Police |
| Chin Han | Councilman Yen |
| Chris Evans | Steve Rogers / Captain America |
| Chris Jameson | DC Businessman |
| Christina Shaffer | DC Driver |
| Christopher George Sarris | Skinny Steve |
| Christopher Kaczmarek | Museum Guest |
| Christopher Markus | S.H.I.E.L.D. Interrogator #1 |
| Christopher Warner | Baseball Coach |
| Cobie Smulders | Agent Maria Hill |
| Colin Botts | DC Pedestrian |
| Cristee Brianas | Mall Guest |
| Cullen G. Chambers | Secretary of Defense |
| Cullum Andrews | Museum Kid |
| D.C. Pierson | Apple Employee |
| Damon Driver | Sergeant Duffy |
| Dan Anders | DC Cop |
| Dan Anders | Driver |
| Danea Rhodes | Mall Pedestrian |
| Daniel Clifford | S.H.I.E.L.D. Strike Agent |
| Danny Pudi | Com Tech #1 |
| Dante Rosalina | Little Boy in the Smithsonian |
| David Biedrzycki | French Mercenary Soldier |
| David Cohen | DC Businessman |
| David Gragg | Museum Patron |
| David Hill | Politician |
| Davis Aguila | S.H.I.E.L.D. Strike Agent |
| Dean Barlage | S.H.I.E.L.D. Agent |
| Debbie Scaletta | Museum Visitor |
| Derek Hughes | Human Resources Executive |
| Derek Talib | S.H.I.E.L.D. Agent |
| Diedra Arthur-O'Ree | Pedestrian |
| Domaine Javier | ER Nurse |
| Dominic Rains | CIA Instructor |
| Dominique Henderson | Pedestrian |
| Dot Gregory | Museum Staff |
| Drew Breeden | Armed Guard |
| Dyrell Barnett | S.H.I.E.L.D. Strike Agent |
| Earl Rorer | Military Veteran |
| Ed Brubaker | Scientist #2 |
| Eddie J. Fernandez | Strike Agent |
| Edward Pfeifer | Mall Patron |
| Elizabeth Olsen | Wanda Maximoff / Scarlet Witch |
| Emerson Brooks | Senior S.H.I.E.L.D. Agent |
| Emily VanCamp | Sharon Carter / Kate / Agent 13 |
| Ethan Rains | Lead EMT |
| Evan Parke | S.H.I.E.L.D. Agent |
| Frank Grillo | Brock Rumlow |
| Gabriella Sagnes | Mall Shopper |
| Gabriella Sagnes | Museum Guest |
| Garry Shandling | Senator Stern |
| Gary Sinise | The Smithsonian Narrator |
| George Ludden | Smithsonian Employee |
| Georges St-Pierre | Georges Batroc |
| Giles Clarke | S.H.I.E.L.D. Strike Agent |
| Griff Allen | Strike Sergeant #2 |
| Guy Cusson | Virtual Repelling Strike Force Agent |
| Hamilton Ray Hodge | S.H.I.E.L.D. Agent |
| Hayley Atwell | Peggy Carter |
| Henry Goodman | Dr. List |
| Inder Kumar | DC Pedestrian |
| J. Blakemore | S.H.I.E.L.D. Agent |
| James Howard | Smithsonian Guard |
| James Lewis | Smithsonian Museum Visitor |
| Jasmine With | Mall Patron |
| Jason G. Sarris | S.H.I.E.L.D. Agent |
| Jason Klingensmith | S.H.I.E.L.D. Agent |
| Jason L. Wang | DC Pedestrian |
| Jason Rocco | Museum Visitor |
| Jason Speer | Husband |
| Jeff Seich | S.H.I.E.L.D. Security Guard |
| Jenna Hoskins | DC Business Woman |
| Jennifer Lavi | DC Business Woman |
| Jenny Agutter | World Security Councilwoman Hawley |
| Jenny Agutter | Natasha Romanoff / Black Widow as Councilwoman Hawley |
| Jeremy Maxwell | Lead S.H.I.E.L.D. Pilot |
| Jeremy Michael Burns | S.H.I.E.L.D. Strike Agent |
| Jimmel Young | Mall Pedestrian |
| JoAnna Leigh Gerondale | S.H.I.E.L.D. Agent |
| Jody Hart | 25th Floor Strike Agent |
| Joe Rosalina | Strike Agent |
| Joe Russo | Dr. Fine |
| Joel Cole | S.H.I.E.L.D. Flight Deck crew |
| Joel Shock | S.H.I.E.L.D. Security |
| Joel Thingvall | Museum Visitor |
| John Brooks Jr. | Quinjet Pilot |
| John Fecek | DC Professional |
| Johnathon L. Jackson | Strike Force Agent |
| Jon Sklaroff | Charlie XO |
| Jordan Greytak | Military Veteran |
| Jose W. Byers | S.H.I.E.L.D. Strike Agent |
| Joseph McCaughtry | Pedestrian |
| Josh Heileman | S.H.I.E.L.D. Strike Agent |
| Jostein Sagnes | Kid at the museum |
| June Christopher | S.H.I.E.L.D. Computer |
| Justin Lally | Man with Captain America shirt |
| Justin Mitchiner | Apple Employee |
| Karen Gadson Alexander | ER Nurse |
| Katana Ren | DC Pedestrian |
| Kathryn Bright | Museum Visitor |
| Kayla McDonald | Pedestrian |
| Kayla McDonald | Precision Driver |
| Kelly Fandrey | D.C. Pedestrian |
| Ken Bray | Smithsonian Guard |
| Kevin Kissig | Driver |
| Kevin Kissig | S.H.I.E.L.D. Strike Agent |
| Kevin Slone | DC Pedestrian |
| Kris Leiter | Precision Driver |
| Kristen Lee Smith | Museum Guest |
| Kristina Randjelovic | Mall Patron |
| Kristina Randjelovic | S.H.I.E.L.D. Agent |
| Kriz Chris Henri Harriz | Street Dealer |
| LaTrallo Presley | DC Construction Worker |
| LaTrallo Presley | Pedestrian |
| Lauren Gabbard | DC Pedestrian |
| Lawrence Whitener | SAG Vehicle Driver |
| Layla Cushman | S.H.I.E.L.D. Agent |
| Les Mahoney | Quinjet Pilot |
| Logan Fry | Guest Services Volunteer |
| Lucas Lind | CIA Recruit |
| Lynda Santa | DC Pedestrian |
| Mark Falvo | Museum Visitor |
| Marse Ratliff | Businessman |
| Marse Ratliff | Pedestrian |
| Martin Cremer | S.H.I.E.L.D. Agent |
| Martin Reese | S.H.I.E.L.D. Agent |
| Matthew Skomo | S.H.I.E.L.D. Strike Agent |
| Maximiliano Hernández | Agent Jasper Sitwell |
| Melissa Santiago | Mall Patron |
| Michael De Geus | FBI Agent |
| Michael Debeljak | Strike Agent |
| Michael Eric | S.H.I.E.L.D. Strike Agent |
| Michael Simpson Jr. | S.H.I.E.L.D. Agent |
| Michael V. Chastain | Driver |
| Mike Karban | S.H.I.E.L.D. Security Guard |
| Mitchell Yee | HYDRA Soldier |
| Nate Hatton | DC Businessman |
| Neal McNeil | S.H.I.E.L.D. Agent |
| Nestor Serrano | Committee General |
| Nicholas Gibeault | Apple Store Shopper |
| Nicolas Bosc | French Pirate |
| Nicole Tubbs | DC Pedestrian |
| Orion Hughes | D.C. Businessman |
| Orlando McNary | Colonel |
| Pat Healy | Scientist #1 |
| Patrick Michael Strange | DC Businessman |
| Paul David Roberts | Sound Guy |
| Paul J. Porter | S.H.I.E.L.D. Strike Agent |
| Paul Nandzik | Mall Patron |
| Phil Mallon | DC Pedestrian |
| Philip Greene | Smithsonian Visitor |
| Philip Ongert | Ship Hostage |
| Rachel Camacho | Museum Visitor |
| Rachel Herrick | Mall Pedestrian |
| Raiden Integra | Mall Pedestrian |
| Ricardo Chacon | Strike Sergeant #1 |
| Richard M. Hooper | Washington D.C. Pedestrian |
| Rick Dremann | DC Pedestrian |
| Rick L. Dean | Surgeon |
| Robert B. Schneider IV | S.H.I.E.L.D. Agent |
| Robert Clotworthy | Fury Car |
| Robert E. Kerr | S.H.I.E.L.D. Agent |
| Robert P. Thitoff | S.H.I.E.L.D. Agent |
| Robert Redford | Alexander Pierce |
| Rod Fielder | Pedestrian |
| Roger Petan | Man Exiting Apartment 1938 Flashback |
| Ron Underdahl | Riley |
| Roshawn Franklin | Virtual DC Cop |
| Rydell Danzie | S.H.I.E.L.D. Strike Agent |
| Rylend Grant | Stabbing Vagrant |
| Sage Porter | S.H.I.E.L.D. Tech |
| Salvator Xuereb | French Pirate #1 |
| Samuel L. Jackson | Nick Fury |
| Sandhya Chandel | S.H.I.E.L.D. Agent |
| Scarlett Johansson | Natasha Romanoff / Black Widow |
| Scott Lockhart | Pedestrian |
| Sebastian Stan | Bucky Barnes / Winter Soldier |
| Shaira Barton | Tourist |
| Shannon Edwards | DC Commuter |
| Sharita Bone | Patron |
| Sharyn Kmieciak | Mall Patron |
| Sharyn Kmieciak | Museum Visitor |
| Shawn Gonzalez | Museum Guest |
| Simmie Terrell | Civilian |
| Stan Lee | Smithsonian Guard |
| Stephen McFeely | S.H.I.E.L.D. Interrogator #2 |
| Steven Culp | Scudder |
| Steven Thomas Capp | Baseball Player |
| Sue Danna Myer | Mall Patron |
| Tara Kodosky | S.H.I.E.L.D. Tech Agent |
| Terence O'Rourke | FBI Agent |
| Terry McConnaughey | Museum-Employee Supervisor |
| Tex Allen | Diplomat |
| Theresa Wylie | Museum Visitor |
| Thomas Kretschmann | Baron Wolfgang von Strucker |
| Thomas R. Baker | Soldier |
| Toby Jones | Dr. Arnim Zola |
| Tom Shafer | Mall Patron |
| Tony Moore | DC Professional |
| Travis Allen Bush | S.H.I.E.L.D. Agent |
| Travis Wong | French Pirate |
| Travis Wong | S.H.I.E.L.D. Strike Agent |
| Trent Rowland | 1940's Soldier |
| Troy Bogdan | Mall Pedestrian |
| Ulysses E. Campbell | DC Businessman |
| Vimalraj Jayaseelan | Museum Visitor |
| Vincent Riviezzo | DC Businessman |
| Wendy Hoopes | Doctor |
| Xavier Wolf | Boy in Captain America Suit |
| Zack Duhame | Engine Pirate |
